Ask Anton at Rent-a-Tiger in Barcelona, which is by ran the best destination for flights within Europe as well as hosting long haul from wherever ...
Speaking of either France or Spain is a bit meaningless, as to get the best out of the Pyrenees you criss-cross over the border constantly, crossing the frontier several times in the same day. Having said that accommodation, food and even fuel are considerable cheaper in Spain - and it's much more sunny!
Check out my blog for some ideas.
Regs
Simon
PS don't bother with Andorra!
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