Hi,
Message from a "Insider". The route you marked seems to me 99% optimal. IMO I would change the last part from Puigcerdà to Perpinyà by Puigcerdà, Ribes de Fresser, Molló.
Additionally, if your are not planning to buy anything in Andorra, the roads overthere are crazy crowded, almost always 50km/h limited and doesn't make sense.
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