I've been putting places on Destinations. Hit me up when you reach Estonia, or let me know what kind of stuff you're interested in.
Lithuania - the Curonian Spit is normally interesting but otherwise going that far west might not be worthwhile. Have a look at the Hill of Crosses as far as countryside destinations go. Vilnius is a worthwhile stop, but I'm biased since I have friends there.
Latvia - well there's Riga, and lots of nice countryside as well. Some old castles, for example Jaunpils, the seat of Jacob Keller, the Duke of Courland (a very interesting historical person who founded Latvian colonies in Africa and the Caribbean). The Sigulda/Turaida area and Cesis are quite scenic.
Estonia - depends whether you go via the western road (through Pärnu) or the eastern road (through Tartu). I'm more familiar with the eastern road and can give you more tips about that. Definitely go to the islands, Saaremaa and Hiiumaa, if you're camping.
https://loodusegakoos.ee/where-to-go/search-options <<< Nature points of interest in Estonia. Wild camping is allowed, but the national forestry service maintains trails, forest huts and campsites too.
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