Definitely the Picos de Europa is one of the most beautiful areas in Spain to ride. Mountains, beautiful scenery and delicious food (unless you are vegetarian). The Picos are in Asturias and not the same thing as Galicia, which is further east, but very close. It also deserves a loop and North of Portugal. In Galicia roads are worse, but not terrible. And on top of that it is not as hot as the rest of the peninsula in summer.
Enjoy yourself.
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