What are "must see" destinations? It depends what you are interested in. As you have mentioned dirt roads, I'll assume that you care for nature more than culture or history.
Slovenia: Vršić pass, Bled Lake, Postojna cave
Croatia: Backroads in Istria, Mt. Učka, Mt. Velebit with countless dirt roads, Adriatic road between Rijeka and Zadar, Plitvice lakes, Krka waterfalls, Mt. Biokovo,
Croatia/Bosnia: Željava deserted air base (partly in Croatia), take care not to unintentionally get out of EU illegally. If you go there, climb to Mt. Plješivica.
Bosnia: River Una canyon, Kravice waterfalls, the springs of river Bosnia in Sarajevo-Ilidža, and river Buna in Blagaj, the old forest Peručica - plenty of unpaved roads everywhere.
Montenegro: Mt Durmitor, The canyon of river Tara, The bay of Kotor, Lake Skadar, the mouth of river Bojana
Serbia: Zlatibor, Đerdap gorge, Ibar canyon, Mt Kopaonik
Romania: Transfagarasan, Transalpina,
the list goes on and on and on...
Some border crossings are just for locals, but those are not on any maps.
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